A novel microwave-assisted methanol-to-hydrocarbons process with a structured ZSM-5/SiC foam catalyst: Proof-of-concept and environmental impacts
نویسندگان
چکیده
This study presents a novel combination of microwave irradiation and structured zeolite/SiC foam catalyst to improve the methanol-to-hydrocarbons (MTH) process as well its environmental sustainability. Accordingly, ZSM-5/SiC was studied under at various reaction temperatures (400–550 °C) space velocities (8 12 h−1) compared conventional ZSM-5 pellets. promoted higher selectivity towards C1−C5 hydrocarbons (∼95%) particularly propylene (∼40% 400 °C 8 pellets 6–9%, respectively) due enhanced mass heat transfers. The microwave-assisted MTH with both also assessed on sustainability via life cycle assessment in comparison conventionally-heat catalyst. results showed that microwave-based could reduce impacts production by 22–30% conventionally-heated same
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Please note that technical editing may introduce minor changes to the text and/or graphics, which may alter content. The journal’s standard Terms & Conditions and the Ethical guidelines still apply. In no event shall the Royal Society of Chemistry be held responsible for any errors or omissions in this Accepted Manuscript or any consequences arising from the use of any information it contains. ...
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ژورنال
عنوان ژورنال: Chemical Engineering Science
سال: 2022
ISSN: ['1873-4405', '0009-2509']
DOI: https://doi.org/10.1016/j.ces.2022.117669